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Hardcover - 9789811007729
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Beschreibung
This thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd–Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD). The excellent correlation between model surfaces and supported catalysts demonstrates the feasibility of designing effective bimetallic catalysts for selective hydrogenation reactions. The author also proposes a method for designing non-precious metal catalysts to replace precious metals. She modifies the process of selective hydrogenation of acetylene by coupling the selective adsorption to the selective hydrogenation in the liquid phase, as a result of which the ethylene selectivity is greatly improved and heat transfer is greatly enhanced. Lastly, by analyzing the mechanism of liquid-phase hydrogenation, the author proposes a multi-stage slurry bed reactor for industrial applications.<
Details
| Verlag | Springer Singapore |
| Ersterscheinung | 07. Juli 2018 |
| Maße | 23.5 cm x 15.5 cm |
| Gewicht | 248 Gramm |
| Format | Softcover |
| ISBN-13 | 9789811092473 |
| Auflage | Softcover reprint of the original 1st edition 2017 |
| Seiten | 141 |
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